Kieron Burke, Neepa Maitra,
and Ivo Souza
Dept of Chemistry and Chemical Biology and
Dept of Physics and Astronomy, Rutgers University
In 1995, Gonze, Ghosez, and Godby, showed that the periodic density in a bulk
insulator in an external electric field does not uniquley determine the external
potential, leading to an ultra-nonlocal dependence of the macroscopic exchange-correlation
electric field on the density. By considering the situation from a time-dependent
viewpoint, we explain the origin of this effect and show why the current-density
is the appropriate variable for describing this phenomenon. No ultra-nonlocality
is needed in a time-dependent current density functional theory.